Characters that are considered to be heroes, which includes police officers and other heroes.
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- Saint Joseph
- Sam (barfly)
- Scratchy
- Scratchy Jr.
- Jay Sherman
- Simpson family
- Bart Simpson
- Cyrus Simpson
- Eliza Simpson
- Homer Simpson
- Lisa Simpson
- Mabel Simpson
- Maggie Simpson
- Marge Simpson
- The Simpsons
- Sheldon Skinner
- Wayne Slater
- Sara Sloane
- Waylon Smithers, Jr.
- Waylon Smithers, Sr.
- Stegosaurus
- Strangles